I’m not specifically knowledgeable about Rydberg polaritons, but in general, it’s not that something is switching between light and matter, but that the material allows / enforces a condition where light passing through interacts with the crystal in a way that generates some kind of atomic motion or electron behavior, like maybe a compression wave, etc., which then also changes the way the light moves (like index of refraction).
The result is it’s not easy to do the math for the light alone, since it’s so heavily influenced by the atoms, and you also can’t easily do the math for the atomic behavior.
But if you’re willing to give up the idea that the light and crystal are different things, you can combine the equations in a way where there’s no simple way to work with just light or just atoms, but easy to work with a new type of thing (polariton) that behaves like a discreet object that flies through the crystal like it’s in free space. And polaritons interact with each other like they’re simple particles instead of giant complex, spread out combinations of light waves and atomic oscillations.
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